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Electrochemiluminescence Imaging-Based High-Throughput Screening Platform for Electrocatalysts Used in Fuel Cells

机译:基于电化学发光成像的高通量筛选平台,用于燃料电池中的电催化剂

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摘要

High throughput screening is very important for accelerating the discovery of fuel cell catalysts. In this paper, a novel electrochemiluminescence (ECL, a technology changing electric current into light) imaging-based screening platform for electrocatalysts used in fuel cells has been developed. The ECL imaging-based screening platform consists of bipolar electrode array-bridged electrochemical (EC)/ECL twin cells, by which electrocatalytic reduction currents of O_(2) can be imaged directly by ECL. The ECL imaging-based screening platform is simple in instrumentation, can image the "current-voltage" dependence directly, reversibly, and sensitively, and may enable the activities of electrocatalysts to be evaluated in a high-throughput way. The developed ECL imaging-based screening platform is envisioned to have promising applications in high throughput combinatorial screening of electrocatalysts for fuel cells.
机译:高通量筛选对于加速燃料电池催化剂的发现非常重要。在本文中,已开发出一种基于新型电化学发光(ECL,一种将电流转换为光的技术)成像的燃料电池电催化剂筛选平台。基于ECL成像的筛选平台由双极电极阵列桥式电化学(EC)/ ECL双胞胎组成,通过该双电池,ECL可以直接成像O_(2)的电催化还原电流。基于ECL成像的筛选平台仪器简单,可以直接,可逆和敏感地对“电流-电压”依赖性进行成像,并且可以以高通量方式评估电催化剂的活性。预计开发的基于ECL成像的筛选平台将在燃料电池电催化剂的高通量组合筛选中具有广阔的应用前景。

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