Gold-Catalyzed Tandem Cycloisomerization-Halogenation of Chiral Homopropargyl Sulfonamides

Shu Chao; Li Long; Shen Cang-Hai; Ruan Peng-Peng; Liu Chao-Yue; Ye Long-Wu

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Gold-Catalyzed Tandem Cycloisomerization-Halogenation of Chiral Homopropargyl Sulfonamides

机译：金催化手性高炔丙基磺酰胺的串联环化异构化反应

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Two new gold-catalyzed tandem cycloisomerization-halogenation reactions of chiral homopropargyl sulfonamides have been developed. Various enantioenriched 3,3-diiodopyrrolidin-2-ols and 3-fluoropyrrolidin-2-ols were obtained in moderate-to-good yields with excellent enantio- and diastereoselectivity.

机译：已经开发了两个新的手性高炔丙基磺酰胺的金催化的串联环异构化-卤化反应。以中等至良好的产率获得了各种对映体富集的3,3-二碘吡咯烷醇-2-醇和3-氟吡咯烷酮-2-醇，具有优异的对映体和非对映体选择性。

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《Chemistry: A European journal》 |2016年第7期|共9页
作者
Shu Chao; Li Long; Shen Cang-Hai; Ruan Peng-Peng; Liu Chao-Yue; Ye Long-Wu;
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正文语种 eng
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cycloisomerization; gold; halogenation; heterocycles; homogeneous catalysis;

机译：环异构化;金;卤化;杂环;均相催化;

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专利

1. Gold-Catalyzed Tandem Cycloisomerization-Halogenation of Chiral Homopropargyl Sulfonamides [J] . Shu Chao, Li Long, Shen Cang-Hai, Chemistry: A European journal . 2016,第7期

机译：金催化手性高炔丙基磺酰胺的串联环化异构化反应
2. Gold-Catalyzed Tandem Cycloisomerization and Dimerization of Chiral Homopropargyl Sulfonamides [J] . Yong-Fei Yu, Chao Shu, Cang-Hai Shen, Chemistry, an Asian journal . 2013,第12期

机译：金催化手性高炔丙基磺酰胺的串联环化和二聚
3. Gold-catalyzed intermolecular oxidation of chiral homopropargyl sulfonamides: a reliable access to enantioenriched pyrrolidin-3-ones [J] . Chao Shu, Long Li, Yong-Fei Yu, Chemical Communications . 2014,第19期

机译：金催化的手性高炔丙基磺酰胺的分子间氧化：可靠地获得对映体富集的吡咯烷-3-酮
4. Chirality Transfer in Gold-Catalyzed Carbothiolation of Alkynes [C] . Takuma Sato, Itaru Nakamura, Masahiro Terada Symposium on Organometallic Chemistry . 2008

机译：金催化碳钙质碳钙质的手性转移
5. Part I: Total Synthesis of (+/-)-Pallambins C and D, and, Part II: Gold-Catalyzed Tandem Cyclization towards Substituted Bicyclo[3.2.1]Octenone Derivatives: Lead to Total Synthesis of Dhilirolides A-D. [D] . Xu, Xuesong. 2013

机译：第一部分：（+/-）-戊二烯C和D的全合成，第二部分：金催化的串联环化反应取代双环[3.2.1]大黄酮衍生物：导致Dhilirolides A-D的全合成。
6. Correction to Chiral Brønsted Acid Catalyzed Enantioselective Synthesis ofanti-Homopropargyl Alcohols via Kinetic Resolution-Aldehyde Allenylboration Using RacemicAllenylboronates [O] . Andy S. Tsai, Ming Chen, William R. Roush -1

机译：手性布朗斯台德酸催化对映体的对映选择性合成消旋动力学拆分醛丙炔基硼酸酯制备抗同炔丙基醇烯丙基硼酸酯
7. Gold-Catalyzed Tandem Cycloisomerizationand Dimerization of Chiral Homopropargyl Sulfonamides [O] . Yong-FeiYu, ChaoShu, Cang-Hai Shen, 2013

机译：金催化手性高炔丙基磺酰胺的串联环化和二聚

Gold-Catalyzed Tandem Cycloisomerization-Halogenation of Chiral Homopropargyl Sulfonamides

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