An improved numerical method to compute neutron/gamma deexcitation cascades starting from a high spin state

摘要

Numerous nuclear processes involve the deexcitation of a compound nucleus through the emission of several neutrons, gamma-rays and/or conversion electrons. The characteristics of such a deexcitation are commonly derived from a total statistical framework often called "Hauser Feshbach" method. In this work, we highlight a numerical limitation of this kind of method in the case of the deexcitation of a high spin initial state. To circumvent this issue, an improved technique called the Fluctuating Structure Properties (FSP) method is presented. Two FSP algorithms are derived and benchmarked on the calculation of the total radiative width for a thermal neutron capture on U-238. We compare the standard method with these FSP algorithms for the prediction of particle multiplicities in the deexcitation of a high spin level of Ba-143. The gamma multiplicity turns out to be very sensitive to the numerical method. The bias between the two techniques can reach 1.5 gamma/cascade. Finally, the uncertainty of these calculations coming from the lack of knowledge on nuclear structure is estimated via the FSP method. (C) 2016 Elsevier B.V. All rights reserved.