Correction for neutron self-shielding in large-sample prompt-gamma neutron activation analysis: Determination of macroscopic neutron cross sections

摘要

When a sample is analysed with neutron activation analysis (NAA) neutron self-shielding and gamma self-absorption affect the accuracy. Both effects become even more important when the mass of a sample analysed is changed from small (say, 1 g) to large (say 30 kg). Therefore, corrections have to be carried out in this article only the correction method for neutron self-shielding is considered for a thermal neutron beam irradiating large homogeneous samples for prompt-gamma NAA (PGNAA). The correction method depends on the macroscopic scattering and absorption cross sections of the sample. To avoid doing experiments with samples with different macroscopic scattering and absorption cross sections, the Monte Carlo model MCNP is applied in the development of the correction method. The computational development of the method to determine these cross sections through flux monitoring outside the sample is described.