This article considers the validity of the coincidence site lattice classification in grain boundary engineering in light of the fact that the coincidence site lattice∑ designation does not directly specify the crystallography at the boundaryplane itself The coincidence site lattice approach is overviewed by reporting selected parts of a recent large-scale survey of experiments on polycrystals that invoke a coincidence site lattice analysis. Second, results from pure nickel are presented that show how a population of grain boundaries can evolve via a fine tuning mechanism recognized by decreasing deviations from exact coincidence site lattice matching.
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