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Non-Hermitian Quantum Mechanics for High-Order Hamronic Generation Spectra

机译:高阶谐波产生谱的非埃尔米特量子力学

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High-order harmonic generation spectra of atoms and molecules in intense laser fields show a wide plateau of odd harmonics, with photon energies high up to the soft X-ray regime. The mechanism leading to the absence of other frequencies, so-called hyper-Raman lines or sidebands, is still unclear. By the user of non-Hermitian quantum mechanics for the many-electron atomic/molecular Hamiltonian system, we derive closed-form expression for the high-order harmonic generation spectra. The analysis of these expressions provides the (already known) conditions for which the hyper-Raman lines are missing and also the conditions for which they are observable. The new information obtained here is proof that in order to observe disbands it is not sufficient to populate two different Floquet states. When the duration of the laser pulse is sufficiently long, the two resonance Floquet states should have similar widths (inverse lifetimes). For short pulses, the condition for observable sidebands is more complicated, and it does not depend directly on the lifetime of the resonance states. By numerical integration of the conventional time-dependent Schrodinger equation, we provide illustrative examples that confirm our conclusions. Our results can be used to design new experiments that will show that fingerprints of the hyper-Raman lines.
机译:在强激光场中原子和分子的高次谐波产生光谱显示出一个宽泛的奇数谐波平台,光子能量高达软X射线状态。导致缺乏其他频率(所谓的超拉曼线或边带)的机制仍不清楚。通过多电子原子/分子哈密顿系统的非赫米特量子力学的用户,我们导出了高次谐波产生谱的闭式表达式。对这些表达式的分析提供了超拉曼谱线缺失的(已知的)条件以及可观察到的条件。此处获得的新信息证明,为了观察解散,不足以填充两个不同的Floquet状态。当激光脉冲的持续时间足够长时,两个共振浮球状态应具有相似的宽度(寿命倒数)。对于短脉冲,可观察边带的条件更加复杂,并且不直接取决于谐振状态的寿命。通过常规时间相关的Schrodinger方程的数值积分,我们提供了例证性的例子来证实我们的结论。我们的结果可用于设计新实验,这些实验将显示超拉曼线条的指纹。

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