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Modelling and simulation of aerosol formation by heterogeneous nucleation in gas-liquid contact devices

机译:气液接触装置中异相成核形成气溶胶的建模与模拟

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摘要

This paper describes a new simulation tool for the prediction of aerosol formation and behaviour in gas-liquid contact devices such as absorbers, scrubbers, quench coolers, and condensers as well as multistage gas cleaning processes, respectively. Aerosol formation can impact severely the separation efficiency of gas cleaning processes. Aerosol or fog formation can arise by spontaneous condensation or desublimation in supersaturated gas phases. The rigorous description of the mass and energy transfer between the gas phase, the liquid phase, and the growing aerosol droplets leads to a system of partial differential and algebraic equations. For the solution of these systems, we have developed the plant simulation tool AerCoDe. This programme bases upon the linearly-implicit Euler discretization, which in combination with extrapolation permits an adaptive step size and order control. Typical simulation results of a multistage industrial flue gas scrubbing process are presented. It is shown, that experimental data can be confirmed if the number concentration of condensation nuclei as an input parameter is roughly known. (C) 2002 Elsevier Science Ltd. All rights reserved. [References: 45]
机译:本文介绍了一种新的模拟工具,用于预测气液接触装置(例如吸收器,洗涤器,骤冷器和冷凝器)中的气溶胶形成和行为,以及多级气体净化过程。气溶胶的形成会严重影响气体净化过程的分离效率。气溶胶或雾气的形成可能是由于过饱和气相中的自然冷凝或升华而引起的。对气相,液相和不断增长的气溶胶液滴之间的质量和能量转移的严格描述导致了偏微分和代数方程组。对于这些系统的解决方案,我们开发了工厂仿真工具AerCoDe。该程序基于线性隐式Euler离散化,结合外推可进行自适应步长和顺序控制。给出了多级工业烟气洗涤过程的典型模拟结果。结果表明,如果以凝结核的数目浓度作为输入参数大致已知,则可以确认实验数据。 (C)2002 Elsevier ScienceLtd。保留所有权利。 [参考:45]

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