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Linewidths in excitonic absorption spectra of cuprous oxide

机译:氧化亚铜的激子吸收光谱中的线宽

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摘要

We present a theoretical calculation of the absorption spectrum of cuprous oxide (Cu2O) based on the general theory developed by Y. Toyozawa. An inclusion not only of acoustic phonons but also of optical phonons and of specific properties of the excitons in Cu2O like the central-cell corrections for the 1S exciton allows us to calculate the experimentally observed linewidths in experiments by T. Kazimierczuk et al. [T. Kazimierczuk, D. Frohlich, S. Scheel, H. Stolz, and M. Bayer, Nature (London) 514, 343 (2014)] within the same order of magnitude, which demonstrates a clear improvement in comparison to earlier work on this topic. We also discuss a variety of further effects, which explain the still observable discrepancy between theory and experiment but can hardly be included in theoretical calculations.
机译:我们根据丰泽(Y.Toyozawa)提出的一般理论介绍了氧化亚铜(Cu2O)吸收光谱的理论计算。在Cu2O中不仅包含声子,还包含光学声子和激子的特定性质,例如1S激子的中心单元校正,使我们能够计算T. Kazimierczuk等人在实验中观察到的线宽。 [T. Kazimierczuk,D。Frohlich,S。Scheel,H。Stolz和M. Bayer,Nature(London)514,343(2014)]处于相同的数量级,与先前在该主题上的工作相比,它显示出明显的改进。我们还将讨论各种进一步的影响,这些影响解释了理论与实验之间仍可观察到的差异,但几乎不能包含在理论计算中。

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