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Improved zircon fission-track annealing model based on reevaluation of annealing data

机译:基于退火数据再评估的改进锆石裂变径迹退火模型

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摘要

The thermal recovery (annealing) of mineral structure modified by the passage of fission fragments has long been studied by the etching technique. In minerals like apatite and zircon, the annealing kinetics are fairly well constrained from the hour to the million-year timescale and have been described by empirical and semi-empirical equations. On the other hand, laboratory experiments, in which ion beams interact with minerals and synthetic ceramics, have shown that there is a threshold temperature beyond which thermal recovery impedes ion-induced amorphization. In this work, it is assumed that this behavior can be extended to the annealing of fission tracks in minerals. It is proposed that there is a threshold temperature, T 0, beyond which fission tracks are erased within a time t 0, which is independent of the current state of lattice deformation. This implies that iso-annealing curves should converge to a fanning point in the Arrhenius pseudo-space (ln t vs. 1/T). Based on the proposed hypothesis, and laboratory and geological data, annealing equations are reevaluated. The geological timescale estimations of a model arising from this study are discussed through the calculation of partial annealing zone and closure temperature, and comparison with geological sample constraints found in literature. It is shown that the predictions given by this model are closer to field data on closure temperature and partial annealing zone than predictions given by previous models.
机译:长期以来,通过蚀刻技术研究了通过裂变碎片通过而改变的矿物结构的热恢复(退火)。在磷灰石和锆石等矿物中,从小时到百万年的时间尺度,退火动力学受到了很好的约束,并已通过经验和半经验方程式进行了描述。另一方面,离子束与矿物和合成陶瓷相互作用的实验室实验表明,存在一个阈值温度,超过该阈值温度,热回收会阻碍离子诱导的非晶化。在这项工作中,假设这种行为可以扩展到矿物中裂变径迹的退火。提出存在阈值温度T 0,在该阈值温度T 0内,在时间t 0内消除了裂变径迹,这与晶格变形的当前状态无关。这意味着等退火曲线应收敛到Arrhenius伪空间中的扇形点(lnt vs.1 / T)。基于提出的假设以及实验室和地质数据,重新评估了退火方程。通过计算局部退火区和封闭温度,并与文献中发现的地质样本约束条件进行比较,讨论了该研究产生的模型的地质时标估计。结果表明,该模型给出的预测比先前模型给出的预测更接近封闭温度和部分退火带的现场数据。

著录项

  • 来源
    《Physics and Chemistry of Minerals》 |2013年第2期|93-106|共14页
  • 作者单位

    Instituto de Física “Gleb Wataghin” Universidade Estadual de Campinas UNICAMP">(1);

    Instituto de Física “Gleb Wataghin” Universidade Estadual de Campinas UNICAMP">(1);

    Chemical and Materials Sciences Division Pacific Northwest National Laboratory">(2);

    Department of Materials Science and Engineering University of Tennessee">(3);

    Materials Science and Technology Division Oak Ridge National Laboratory">(4);

    Instituto de Física “Gleb Wataghin” Universidade Estadual de Campinas UNICAMP">(1);

  • 收录信息
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    Fission tracks; Annealing models; Critical temperature; Zircon;

    机译:裂变径迹;退火模型;临界温度;锆石;

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