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Thermally induced dispersive optical bistability in silver nanosuspensions produced by pulsed laser ablation method

机译:脉冲激光烧蚀法制备的银纳米悬浮液中的热诱导色散双稳态

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摘要

The thermally induced optical bistability in prepared silver (Ag) nanosuspensions have been studied experimentally, using Fabry-Perot and Mach-Zehnder interferometry methods. Two Ag nanosuspensions of different sizes were produced by different fluences of pulsed laser ablation method in distilled water. The pulsed Nd:YAG laser of 7ns pulse width, 1064nm wavelength and different fluences was employed to produce Ag nanosuspensions. Experimental observations were performed by an ultraviolet-visible-near infrared spectrophotometry. Structure and size of prepared Ag nanoparticles were diagnosed using transmission electron microscope images. Fabry-Perot and Mach-Zehnder interferometry methods were used to carry out the optical bistability process in prepared Ag nanosuspensions. In two considered interferometers, the obtained phase shifts of the hysteresis loops based on the optical bistability are inversely proportional to the nonlinear refractive index of samples and thickness of Ag nanosuspensions cells. Results indicate that the induced thermal effect of the optical bistability can be tuned by modifying parameters such as the nonlinear refractive index and applied interferometry methods. Hence, a desirable situation for the thermo-optical effects of the optical bistability can be easily realized in Ag nanosuspensions.
机译:使用法布里-珀罗(Fabry-Perot)和马赫-曾德尔(Mach-Zehnder)干涉测量法,已通过实验研究了制备的银(Ag)纳米悬浮液中的热诱导光学双稳性。通过不同密度的脉冲激光烧蚀法在蒸馏水中制备了两种不同尺寸的银纳米悬浮液。用7ns脉冲宽度,1064nm波长和不同注量的Nd:YAG脉冲激光制备Ag纳米悬浮液。通过紫外可见近红外分光光度法进行实验观察。使用透射电子显微镜图像诊断制备的Ag纳米颗粒的结构和尺寸。用法布里-珀罗(Fabry-Perot)和马赫-曾德尔(Mach-Zehnder)干涉法在制备的Ag纳米悬浮液中进行光学双稳性过程。在两个考虑的干涉仪中,基于光学双稳性获得的磁滞回线的相移与样品的非线性折射率和Ag纳米悬浮液池的厚度成反比。结果表明,可以通过修改参数(例如非线性折射率和应用的干涉测量方法)来调整诱导的光学双稳态热效应。因此,可以在Ag纳米悬浮液中容易地实现对光学双稳性的热光学效应的理想情况。

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