Development of cube-type SOFC stacks using anode-supported tubular cells

摘要

Tubular SOFCs have shown many desirable characteristics such as high thermal stability during rapid heat cycling and large electrode area per unit volume, which can accelerate to realize SOFC systems applicable to portable devices and auxiliary power units for automobile. So far, we have developed anode-supported tubular SOFCs with 0.8-2 mm diameter using Gd-doped CeO_2 (GDC) electrolyte, NiO-GDC anode and (La, Sr)(Co, Fe)O_3 (LSCF)-GDC cathode. In this study, a newly developed cube-type SOFC stack which consists of three SOFC bundles was designed and examined. The bundle consists of three 2 mm diameter tubular SOFCs and a rectangular shaped cathode support where these tubular cells are arranged in parallel. The performance of the stack whose volume is less than 1 cm~3 was shown to be 2.8 V OCV and over 1 W at 1.6 V under 500℃. Cathode loss factor due to current collection from cathode matrix was also estimated using a proposed model.