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Formaldehyde in Various Forms of Atmospheric Precipitation and Deposition from Highly Urbanized Regions

机译:高度城市化地区各种形式的大气降水和沉积甲醛

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Formaldehyde levels were determined in various forms of atmospheric precipitation (rain, snow, road and roof runoff, throughfall) and deposition (rime, hoarfrost, dew) collected over twelve months at various locations in two large urban agglomerations and along two highways. HCHO was found in 303 of 500 samples analyzed, with concentrations ranging from 0.05 to 10.7mg/dm~3. The results confirmed the significant effect of vehicular traffic on formaldehyde levels in various forms of wet deposition. Correlations of formaldehyde levels with other parameters commonly monitored in precipitation and/or deposition were also examined. No correlation was found between HCHO levels and rain volume. On the other hand, positive correlations were found for hydrogen peroxide, non-sea-salt sulphate, nitrate, ammonia, and total organic carbon (TOC). In addition, the effect of selected meteorological parameters (temperature, wind speed, wind direction, rainfall) on the concentration of formaldehyde in various forms of precipitation and runoff (road runoff, roof runoff, throughfall) was studied. The only correlation found was that between HCHO concentration and daily rainfall.
机译:在十二个月内,在两个大型城市群和两条公路的不同位置收集了各种形式的大气降水(雨,雪,道路和屋顶径流,穿透)和沉积物(霜,白霜,露水)中的甲醛含量。在分析的500个样品中的303个中发现了HCHO,浓度范围为0.05至10.7mg / dm〜3。结果证实了各种形式的湿沉降中车辆交通对甲醛水平的显着影响。还检查了甲醛水平与通常在沉淀和/或沉积过程中监测的其他参数的相关性。在HCHO水平和雨量之间没有相关性。另一方面,发现过氧化氢,非海盐硫酸盐,硝酸盐,氨和总有机碳(TOC)呈正相关。此外,还研究了选定的气象参数(温度,风速,风向,降雨)对各种形式的降水和径流(道路径流,屋顶径流,穿透水)中甲醛浓度的影响。发现的唯一相关性是在HCHO浓度和每日降雨量之间。

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