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A metal-insulator transition study of VO_2 thin films grown on sapphire substrates

机译:蓝宝石衬底上生长的VO_2薄膜的金属-绝缘体过渡研究

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摘要

Vanadium thin films were deposited on sapphire substrates by DC magnetron sputtering and then oxidized in a tube furnace filled with oxygen under different temperatures and oxygen flow rates. The significant influence of the oxygen flow rate and oxidation temperature on the electrical and structural properties of the vanadium oxide thin films were investigated systematically. It shows the pure vanadium dioxide (VO_2) state can only be obtained in a very narrow temperature and oxygen flow rate range. The resistivity change during the metal-insulator transition varies from 0.2 to 4 orders of magnitude depending on the oxidation condition. Large thermal hysteresis during the metal-insulator phase transition was observed during the transition compared to the results in literature. Proper oxidation conditions can significantly reduce the thermal hysteresis. The fabricated VO_2 thin films showed the potential to be applied in the development of electrical sensors and other smart devices.
机译:钒薄膜通过直流磁控溅射沉积在蓝宝石衬底上,然后在充满氧气的管式炉中在不同的温度和氧气流速下被氧化。系统地研究了氧气流量和氧化温度对氧化钒薄膜的电学和结构性能的重大影响。它表明只能在非常窄的温度和氧气流速范围内获得纯二氧化钒(VO_2)状态。金属-绝缘体转变期间的电阻率变化取决于氧化条件,从0.2到4个数量级变化。与文献中的结果相比,在过渡期间观察到金属-绝缘体相变期间的大的热滞。适当的氧化条件可以显着降低热滞。制成的VO_2薄膜具有在电子传感器和其他智能设备的开发中应用的潜力。

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  • 来源
    《Journal of Applied Physics》 |2017年第23期|235102.1-235102.5|共5页
  • 作者单位

    Department of Mechanical Engineering, Virginia Polytechnic Institute and State University, Blacksburg, Virginia 24060, USA;

    Department of Mechanical Engineering, Stony Brook University, Stony Brook, New York 11794, USA;

    Center for Functional Nanomaterials, Brookhaven National Laboratory, Upton, New York 11973, USA;

    Department of Mechanical Engineering, Virginia Polytechnic Institute and State University, Blacksburg, Virginia 24060, USA;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
  • 原文格式 PDF
  • 正文语种 eng
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