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Modeling Regional/urban Ozone And Particulate Matter In Beijing, China

机译:中国北京的区域/城市臭氧和颗粒物模拟

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This paper examines Beijing air quality in the winter and summer of 2001 using an integrated air quality modeling system (Fifth Generation Mesoscale Meteorological Model [MM5]/Community Multiscale Air Quality [CMAQ]) in nested mode. The National Aeronautics and Space Administration (NASA) Transport and Chemical Evolution over the Pacific (TRACE-P) emission inventory is used in the 36- (East Asia), 12- (East China), and 4-km (greater Beijing area) domains. Furthermore, we develop a local Beijing emission inventory that is used in the 4-km domain. We also construct a corroborated mapping of chemical species between the TRACE-P inventory and the Carbon Bond IV (CB-IV) chemical mechanism before the integrated modeling system is applied to study ozone (O_3) and particulate matter (PM) in Beijing. Meteorological data for the integrated modeling runs are extracted from MM5. Model results show O_3 hourly concentrations in the range of 80-159 parts per billion (ppb) during summer in the urban areas and up to 189 ppb downwind of the city. High fine PM (PM_(2.5)) concentrations (monthly average of 75 μg·m~(-3) in summer and 150 ng·m~(-3) inrnwinter) are simulated over the metropolitan and downwind areas with significant secondary constituents. A comparison against available O_3 and PM measurement data in Beijing is described. We recommend refinements to the developed local Beijing emission inventory to improve the simulation of Beijing's air quality. The 4-km modeling configuration is also recommended for the development of air pollution control strategies.
机译:本文采用集成的空气质量建模系统(第五代中尺度气象模型[MM5] /社区多尺度空气质量[CMAQ])以嵌套模式研究了2001年冬季和夏季的北京空气质量。美国国家航空航天局(NASA)的太平洋运输和化学演化(TRACE-P)排放清单用于36-(东亚),12-(华东)和4-km(更大的北京地区)域。此外,我们开发了在4公里范围内使用的北京当地排放清单。在集成模型系统用于研究北京的臭氧(O_3)和颗粒物(PM)之前,我们还建立了TRACE-P库存与碳键IV(CB-IV)化学机理之间化学物种的确证映射。从MM5中提取了用于集成建模运行的气象数据。模型结果显示,夏季市区的O_3每小时浓度在十亿分之80-159的范围内,而在下风向则为189 ppb。在大城市和顺风地区模拟了较高的精细PM(PM_(2.5))浓度(夏季每月平均为75μg·m〜(-3),冬季为150 ng·m〜(-3),次要成分较高。描述了与北京现有O_3和PM测量数据的比较。我们建议对已开发的北京当地排放清单进行改进,以改善对北京空气质量的模拟。还建议使用4公里的建模配置来制定空气污染控制策略。

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