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Lasing in dark and bright modes of a finite-sized plasmonic lattice

机译:在黑暗和明亮的模式下激化有限尺寸的等离激元晶格

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摘要

Lasing at the nanometre scale promises strong light-matter interactions and ultrafast operation. Plasmonic resonances supported by metallic nanoparticles have extremely small mode volumes and high field enhancements, making them an ideal platform for studying nanoscale lasing. At visible frequencies, however, the applicability of plasmon resonances is limited due to strong ohmic and radiative losses. Intriguingly, plasmonic nanoparticle arrays support non-radiative dark modes that offer longer life-times but are inaccessible to far-field radiation. Here, we show lasing both in dark and bright modes of an array of silver nanoparticles combined with optically pumped dye molecules. Linewidths of 0.2?nm at visible wavelengths and room temperature are observed. Access to the dark modes is provided by a coherent out-coupling mechanism based on the finite size of the array. The results open a route to utilize all modes of plasmonic lattices, also the high- Q ones, for studies of strong light-matter interactions, condensation and photon fluids.
机译:纳米级的激光发射保证了强大的光物质相互作用和超快的运行速度。金属纳米粒子支持的等离子共振具有极小的模式体积和高场增强,使其成为研究纳米级激光的理想平台。然而,在可见频率处,由于强烈的欧姆和辐射损耗,等离子激元共振的适用性受到限制。有趣的是,等离激元纳米颗粒阵列支持非辐射暗模式,该模式可提供更长的使用寿命,但远场辐射无法到达。在这里,我们展示了与光泵浦染料分子结合的银纳米颗粒阵列在黑暗和明亮模式下的激光发射。可见波长和室温下的线宽为0.2?nm。通过基于阵列的有限大小的相干输出耦合机制,可以访问暗模式。研究结果为利用等离子激元晶格的所有模式以及高Q晶格开辟了一条途径,用于研究强光-物质相互作用,凝聚和光子流体。

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