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Circuit Model of Plasmon-Enhanced Fluorescence

机译:等离子体增强荧光的电路模型

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Hybridized decaying oscillations in a nanosystem of two coupled elements—a quantum emitter and a plasmonic nanoantenna—are considered as a classical effect. The circuit model of the nanosystem extends beyond the assumption of inductive or elastic coupling and implies the near-field dipole-dipole interaction. Its results fit those of the previously developed classical model of Rabi splitting, however going much farther. Using this model, we show that the hybridized oscillations depending on the relationships between design parameters of the nanosystem correspond to several characteristic regimes of spontaneous emission. These regimes were previously revealed in the literature and explained involving semiclassical theory. Our original classical model is much simpler: it results in a closed-form solution for the emission spectra. It allows fast prediction of the regime for different distances and locations of the emitter with respect to the nanoantenna (of a given geometry) if the dipole moment of the emitter optical transition and its field coupling constant are known.
机译:两个耦合元素(量子发射器和等离子体纳米天线)的纳米系统中的混合衰减振荡被认为是经典效应。纳米系统的电路模型超出了电感耦合或弹性耦合的假设,并暗示了近场偶极-偶极相互作用。其结果与先前开发的Rabi分裂经典模型的结果相符,但是效果要远得多。使用该模型,我们表明取决于纳米系统设计参数之间的关系的杂交振荡对应于自发发射的几种特征机制。这些制度先前已在文献中揭示,并涉及半古典理论进行了解释。我们最初的经典模型要简单得多:它为发射光谱提供了一种封闭形式的解决方案。如果已知发射器光学跃迁的偶极矩及其场耦合常数,则可以快速预测发射器相对于(给定几何形状)纳米天线的不同距离和位置的状态。

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