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Broadband spontaneous emission rate enhancement through the design of plasmonic nanoantennas

机译:通过设计等离子纳米天线提高宽带自发发射速率

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We numerically investigate and experimentally demonstrate a new route to controllably manipulate the spontaneous decay rate of dipole emitters in coupled plasmonic modes. The structure under investigation is an hexagonal close-packed array of gold core - silica shell nanoparticles (NPs) sandwiched between two gold films. We show that the interaction of localized and propagating surface plasmon polaritons can dramatically enhance the spontaneous emission rate of quantum emitters (rhodamine isothiocyanate) grafted in the NP silica shell. This strong enhancement (70 – 100 times) further occurs on the whole, broadband emission spectrum (565 nm to 640 nm) of the emitters.
机译:我们通过数值研究和实验证明了在耦合等离子体激元模式下可控地控制偶极子发射器自发衰减速率的新途径。正在研究的结构是金芯的六方密堆积阵列-夹在两个金膜之间的二氧化硅壳纳米粒子(NP)。我们表明,局部和传播的表面等离激元极化子的相互作用可以显着提高接枝在NP二氧化硅壳中的量子发射体(罗丹明异硫氰酸盐)的自发发射速率。这种强大的增强作用(70 – 100倍)还发生在发射器的整个宽带发射光谱(565 nm至640 nm)上。

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