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Aerosol emissions factors from traditional biomass cookstoves in India: insights from field measurements

机译:印度传统生物质炊具的气溶胶排放因子:现场测量的见解

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Residential solid biomass cookstoves are important sources of aerosol emissions in India. Cookstove emissions rates are largely based on laboratory experiments conducted using the standard water-boiling test, but real-world emissions are often higher owing to different stove designs, fuels, and cooking methods. Constraining mass emissions factors (EFs) for prevalent cookstoves is important because they serve as inputs to bottom-up emissions inventories used to evaluate health and climate impacts. Real-world EFs were measured during winter 2015 for a traditional cookstove (ichulha/i) burning fuel wood, agricultural residue, and dung from different regions of India. Average (±95?% confidence interval) EFs for fuel wood, agricultural residue, and dung were (1)?PMsub2.5/sub mass: 10.5 (7.7–13.4)?g?kgsup?1/sup, 11.1 (7.7–15.5)?g?kgsup?1/sup, and 22.6 (14.9–32.9)?g?kgsup?1/sup, respectively; (2)?elemental carbon (EC): 0.9 (0.6–1.4)?g?kgsup?1/sup, 1.6 (0.6–3.0)?g?kgsup?1/sup, and 1.0 (0.4–2.0)?g?kgsup?1/sup, respectively; and (3)?organic carbon (OC): 4.9 (3.2–7.1)?g?kgsup?1/sup, 7.0 (3.5–12.5)?g?kgsup?1/sup, and 12.9 (4.2–15.01)?g?kgsup?1/sup, respectively. The mean (±95?% confidence interval) OC?∕?EC mass ratios were 6.5 (4.5–9.1), 7.6 (4.4–12.2), and 12.7 (6.5–23.3), respectively, with OC and EC quantified by the IMPROVE_A thermal-optical reflectance protocol. These real-world EFs are higher than those from previous laboratory-based measurements. Combustion conditions have larger effects on EFs than the fuel types. We also report the carbon mass fractions of our aerosol samples determined using the thermal-optical reflectance method. The mass fraction profiles are consistent between the three fuel categories but markedly different from those reported in past literature – including the source profiles for wood stove PMsub2.5/sub emissions developed as inputs to receptor modeling studies conducted by the Central Pollution Control Board of India. Thermally stable OC (OC3 in the IMPROVE_A protocol) contributed nearly 50?% of the total carbon mass for emissions from all fuels.
机译:家用固体生物质炊具是印度气溶胶排放的重要来源。炉灶的排放率主要基于使用标准开水测试进行的实验室实验,但是由于炉灶设计,燃料和烹饪方法的不同,实际排放量通常更高。限制普遍炊具的质量排放因子(EFs)很重要,因为它们是自下而上的排放清单的输入,用于评估健康和气候影响。在2015年冬季,对来自印度不同地区的传统柴炉( chulha )燃烧的薪柴,农业残留物和粪便的真实EF进行了测量。薪材,农残和粪便的平均EF(置信区间±95%)为(1)?PM 2.5 质量:10.5(7.7–13.4)?g?kg ?1 ,11.1(7.7–15.5)?g?kg ?1 和22.6(14.9–32.9)?g?kg ?1 ; (2)元素碳(EC):0.9(0.6–1.4)?g?kg ?1 ,1.6(0.6–3.0)?g?kg ?1 ,和1.0(0.4–2.0)?g?kg ?1 ; (3)有机碳(OC):4.9(3.2–7.1)?g?kg ?1 ,7.0(3.5–12.5)?g?kg ?1 和12.9(4.2–15.01)?g?kg ?1 。 OC ∕ EC的平均质量比(±95%置信区间)为6.5(4.5-9.1),7.6(4.4-12.2)和12.7(6.5-23.3),其中OC和EC通过IMPROVE_A进行量化热光反射协议。这些实际的EF高于以前基于实验室的测量得出的EF。燃烧条件对EF的影响要大于燃料类型。我们还报告了使用热光反射法确定的气溶胶样品的碳质量分数。这三种燃料的质量分数分布图是一致的,但与以往文献中报道的质量分布图显着不同–包括作为中央污染进行的受体建模研究输入的木灶PM 2.5 排放源分布印度控制委员会。热稳定的OC(IMPROVE_A协议中的OC3)占所有燃料排放碳总量的近50%。

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