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A [NiFe]hydrogenase model that catalyses the release of hydrogen from formic acid

机译：催化从甲酸中释放氢的[NiFe]氢化酶模型

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摘要

We report the decomposition of formic acid to hydrogen and carbon dioxide, catalysed by a NiRu complex originally developed as a [NiFe]hydrogenase model. This is the first example of H_2 evolution, catalysed by a [NiFe]hydrogenase model, which does not require additional energy.
机译：我们报道了由最初作为[NiFe]氢化酶模型开发的NiRu配合物催化的甲酸分解为氢和二氧化碳。这是由[NiFe]氢化酶模型催化的H_2释放的第一个例子，不需要额外的能量。

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  • 来源
    《Chemical Communications》 |2014年第87期|13385-13387|共3页
  • 作者

    Nga T. Nguyen; Yuki Mori; Takahiro Matsumoto; Takeshi Yatabe; Ryota Kabe; Hidetaka Nakai; Ki-Seok Yoon; Seiji Ogo;

  • 作者单位

    Centre for Small Molecule Energy, Kyushu University, 744 Moto-oka,Nishi-ku, Fukuoka 819-0395, Japan,Department of Chemistry and Biochemistry, Graduate School of Engineering,Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan,International Institute for Carbon-Neutral Energy Research (WPI-I2CNER),Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan;

    Department of Chemistry and Biochemistry, Graduate School of Engineering,Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan,International Institute for Carbon-Neutral Energy Research (WPI-I2CNER),Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan;

    Centre for Small Molecule Energy, Kyushu University, 744 Moto-oka,Nishi-ku, Fukuoka 819-0395, Japan,Department of Chemistry and Biochemistry, Graduate School of Engineering,Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan,International Institute for Carbon-Neutral Energy Research (WPI-I2CNER),Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan;

    Centre for Small Molecule Energy, Kyushu University, 744 Moto-oka,Nishi-ku, Fukuoka 819-0395, Japan,Department of Chemistry and Biochemistry, Graduate School of Engineering,Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan,International Institute for Carbon-Neutral Energy Research (WPI-I2CNER),Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan;

    Department of Chemistry and Biochemistry, Graduate School of Engineering,Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan;

    Centre for Small Molecule Energy, Kyushu University, 744 Moto-oka,Nishi-ku, Fukuoka 819-0395, Japan,Department of Chemistry and Biochemistry, Graduate School of Engineering,Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan;

    Centre for Small Molecule Energy, Kyushu University, 744 Moto-oka,Nishi-ku, Fukuoka 819-0395, Japan,International Institute for Carbon-Neutral Energy Research (WPI-I2CNER),Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan;

    Centre for Small Molecule Energy, Kyushu University, 744 Moto-oka,Nishi-ku, Fukuoka 819-0395, Japan,Department of Chemistry and Biochemistry, Graduate School of Engineering,Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan,International Institute for Carbon-Neutral Energy Research (WPI-I2CNER),Kyushu University, 744 Moto-oka, Nishi-ku, Fukuoka 819-0395, Japan;

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