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Polarization switching and electrical control of interlayer excitons in two-dimensional van der Waals heterostructures

机译:二维范德华异质结构中层间激子的极化转换和电控制

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摘要

Long-lived interlayer excitons in van der Waals heterostructures based on transition metal dichalcogenides, together with unique spin-valley physics, make them promising for next-generation photonic and valleytronic devices. While the emission characteristics of interlayer excitons have been studied, efficient manipulation of their valley-state, a necessary requirement for information encoding, is still lacking. Here, we demonstrate comprehensive electrical control of interlayer excitons in a MoSe2/WSe2 heterostructure. Encapsulation of our well-aligned stack with hexagonal boron nitride (h-BN) allows us to resolve two separate narrow interlayer transitions with opposite helicities under circularly polarized excitation, either preserving or reversing the polarization of incoming light. By electrically controlling their relative intensities, we realize a polarization switch with tuneable emission intensity and wavelength. Finally, we demonstrate large Zeeman shifts of these two transitions upon application of an external magnetic field. These results are interpreted within the picture of moiré-induced brightening of forbidden optical transitions. The ability to control the polarization of interlayer excitons is a step forward towards the manipulation of the valley degree-of-freedom in realistic device applications.
机译:基于过渡金属二硫属化物的范德华异质结构中的长寿命层间激子,再加上独特的自旋谷物理学,使其成为下一代光子和谷电子器件的有希望的选择。虽然已经研究了层间激子的发射特性,但是仍然缺乏对谷底态的有效操纵,这是信息编码的必要要求。在这里,我们展示了MoSe2 / WSe2异质结构中层间激子的全面电学控制。用六方氮化硼(h-BN)封装好排列良好的叠层,可以使我们在圆偏振激发下解析两个具有相反螺旋度的单独的窄层间过渡,从而保留或反转入射光的偏振。通过电控制它们的相对强度,我们实现了具有可调发射强度和波长的偏振开关。最后,我们展示了在施加外部磁场时这两个跃迁的大塞曼位移。这些结果在莫尔条纹引起的禁止的光学跃迁变亮的图片中得到了解释。控制层间激子极化的能力是在实际器件应用中朝着操纵谷自由度迈出的一步。

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