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Exploration of laser-driven electron-multirescattering dynamics in high-order harmonic generation

机译:高次谐波产生中激光驱动的电子多散射动力学的探索

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摘要

Multiple rescattering processes play an important role in high-order harmonic generation (HHG) in an intense laser field. However, the underlying multi-rescattering dynamics are still largely unexplored. Here we investigate the dynamical origin of multiple rescattering processes in HHG associated with the odd and even number of returning times of the electron to the parent ion. We perform fully ab initio quantum calculations and extend the empirical mode decomposition method to extract the individual multiple scattering contributions in HHG. We find that the tunneling ionization regime is responsible for the odd number times of rescattering and the corresponding short trajectories are dominant. On the other hand, the multiphoton ionization regime is responsible for the even number times of rescattering and the corresponding long trajectories are dominant. Moreover, we discover that the multiphoton- and tunneling-ionization regimes in multiple rescattering processes occur alternatively. Our results uncover the dynamical origin of multiple rescattering processes in HHG for the first time. It also provides new insight regarding the control of the multiple rescattering processes for the optimal generation of ultrabroad band supercontinuum spectra and the production of single ultrashort attosecond laser pulse.
机译:多次散射过程在强激光场中的高次谐波产生(HHG)中起着重要作用。但是,基本的多重散射动力学仍未得到充分探索。在这里,我们研究了HHG中多次散射过程的动力学起源,该过程与电子返回母离子的奇数和偶数返回次数有关。我们执行从头算起的量子计算,并扩展经验模式分解方法以提取HHG中的各个多重散射贡献。我们发现,隧穿电离机制是造成奇数次散射的原因,而相应的短轨迹占主导地位。另一方面,多光子电离机制负责偶数次散射,并且相应的长轨迹占主导地位。此外,我们发现在多次散射过程中多光子和隧穿电离机制交替出现。我们的结果首次揭示了HHG中多重散射过程的动力学起源。它还为控制多个散射过程提供了新的见识,以最佳地产生超宽带超连续谱并产生单个超短阿秒激光脉冲。

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