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Symmetry-breaking induced magnetic Fano resonances in densely packed arrays of symmetric nanotrimers

机译:密集排列的对称纳米三聚体阵列中的对称性破坏诱导的磁性Fano共振

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摘要

Due to unique properties and great design flexibilities, Fano resonances represent one of the most promising optical features mediated by metallic nanostructures, while the excitation of some Fano modes is impossible due to symmetry reasons. The aim of this work is to show that dense lattice arrangements can have a profound impact on the optical properties of nanostructures and, in particular, can enable the excitation of otherwise dark modes. Here, we demonstrate this concept using the example of rectangular arrays of symmetric trimers packed so densely that the coupling between neighbouring unit cells imposes a symmetry break, enabling the excitation of magnetic Fano resonances. We found that in experiments as well as in simulations, electric and magnetic Fano resonances can be simultaneously formed in cases where the inter-trimer distances are sufficiently small. By analysing the transition from an isolated trimer mode into a regime of strong near-field coupling, we show that by modifying the rectangular unit cell lengths due to the symmetry mismatch between lattice and trimer, two types of Fano resonances can be found, especially magnetic Fano resonances with loop-type magnetic field distributions within the centre of each trimer, which can be either enhanced or suppressed. In addition, the influence of the refractive index environment was measured, showing sensitivity values of approximately 300 nm/RIU. Our work provides fundamental insights into the interaction of the lattice and nanostructure response and paves the way towards the observation of novel optical excitations.
机译:由于独特的性能和出色的设计灵活性,Fano共振代表了由金属纳米结构介导的最有希望的光学特征之一,而由于对称性原因,某些Fano模的激发是不可能的。这项工作的目的是表明致密的晶格排列可以对纳米结构的光学性能产生深远的影响,特别是可以激发其他暗模式的激发。在这里,我们使用密集排列的对称三聚体矩形阵列的示例来演示此概念,以使相邻单位单元之间的耦合强加对称性破坏,从而激发Fano磁共振。我们发现,在实验以及模拟中,在三聚体之间的距离足够小时,可以同时形成电和磁Fano共振。通过分析从孤立的三聚体模式到强近场耦合状态的过渡,我们表明,由于晶格和三聚体之间的对称性不匹配,通过修改矩形晶胞长度,可以发现两种类型的Fano共振,尤其是磁场共振在每个三聚体中心内具有环型磁场分布的法诺共振,可以增强或抑制。此外,测量了折射率环境的影响,显示出大约300 nm / RIU的灵敏度值。我们的工作为了解晶格和纳米结构响应之间的相互作用提供了基本见识,并为观察新型光学激发铺平了道路。

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