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Optical absorbing origin of chiroptical activity in planar plasmonic metasurfaces

机译:平面等离子体亚表面中手性活动的光吸收起源

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摘要

As a significant characteristic of many biomolecules, chemical substances, and artificial nanostructures, chirality conduce different types of optical interactions with the spin angular momentum of the impinging light field. Although, chiral arrangement and spatial phase retardation are the key factors for obtaining chirality in three-dimensional (3D) structures, the origin of chirality in the feasible planar structures has not been thoroughly addressed. Here using an intuitive and simple analytical approach, called cross-hybridization model, the essence and properties of the optical chirality of individual planar nanostructures are unveiled. In order to fundamentally address this chirality in terms of circular dichroism (CD), the chiroptical response of a simple dimer composed of the lossy nanoblocks in L-shape arrangement are investigated based on the provided optical interaction and loss effects. The theoretical findings, adequately supported by the numerical calculations, reveal that chiroptical activity occurs predominantly due to handedness-dependent absorption or heating loss in a nanostructured metasurface.
机译:作为许多生物分子,化学物质和人工纳米结构的重要特征,手性可与入射光场的自旋角动量产生不同类型的光学相互作用。尽管手性排列和空间相位延迟是在三维(3D)结构中获得手性的关键因素,但可行平面结构中手性的起源尚未得到彻底解决。在这里,使用一种称为交叉杂交模型的直观,简单的分析方法,揭示了单个平面纳米结构的光学手性的本质和性质。为了从圆二色性(CD)方面从根本上解决这种手性问题,基于提供的光学相互作用和损失效应,研究了由L型排列的有损纳米嵌段组成的简单二聚体的手性响应。数值计算充分支持的理论发现表明,按摩疗法活动的发生主要是由于纳米结构超表面中依赖于手性的吸收或热损失。

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