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Brownian motion and quantum dynamics of magnetic monopoles in spin ice

机译:旋转冰中磁单极子的布朗运动和量子动力学

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摘要

Spin ice illustrates many unusual magnetic properties, including zero point entropy, emergent monopoles and a quasi liquid–gas transition. To reveal the quantum spin dynamics that underpin these phenomena is an experimental challenge. Here we show how crucial information is contained in the frequency dependence of the magnetic susceptibility and in its high frequency or adiabatic limit. The typical response of Dy2Ti2O7 spin ice indicates that monopole diffusion is Brownian but is underpinned by spin tunnelling and is influenced by collective monopole interactions. The adiabatic response reveals evidence of driven monopole plasma oscillations in weak applied field, and unconventional critical behaviour in strong applied field. Our results clarify the origin of the relatively high frequency response in spin ice. They disclose unexpected physics and establish adiabatic susceptibility as a revealing characteristic of exotic spin systems.
机译:自旋冰说明了许多不寻常的磁特性,包括零点熵,出现的单极子和准的液-气过渡。揭示支撑这些现象的量子自旋动力学是一项实验挑战。在这里,我们显示了关键信息如何包含在磁化率的频率依赖性及其高频或绝热极限中。 Dy2Ti2O7自旋冰的典型响应表明,单极扩散为布朗,但受自旋隧穿的影响,并受集体单极相互作用的影响。绝热响应揭示了在弱应用领域中驱动单极等离子体振荡的迹象,以及在强应用领域中非常规的临界行为。我们的结果阐明了旋转冰中相对较高频率响应的起源。他们揭示了意想不到的物理学,并建立了绝热磁化率作为外来自旋系统的显着特征。

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