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Fractal analysis of collision cascades in pulsed-ion-beam-irradiated solids

机译:脉冲离子束辐照固体中碰撞级联的分形分析

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摘要

The buildup of radiation damage in ion-irradiated crystals often depends on the spatial distribution of atomic displacements within collision cascades. Although collision cascades have previously been described as fractals, the correlation of their fractal parameters with experimental observations of radiation damage buildup remains elusive. Here, we use a pulsed-ion-beam method to study defect interaction dynamics in 3C-SiC irradiated at 100 °C with ions of different masses. These data, together with results of previous studies of SiC and Si, are analyzed with a model of radiation damage formation which accounts for the fractal nature of collision cascades. Our emphasis is on the extraction of the effective defect diffusion length from pulsed beam measurements. Results show that, for both Si and SiC, collision cascades are mass fractals with fractal dimensions in the range of ~1–2, depending on ion mass, energy, and the depth from the sample surface. Within our fractal model, the effective defect diffusion length is ~10 nm for SiC and ~20 nm for Si, and it decreases with increasing cascade density. These results demonstrate a general method by which the fractal nature of collision cascades can be used to explain experimental observations and predict material’s response to radiation.
机译:离子辐照晶体中辐射损伤的积累通常取决于碰撞级联中原子位移的空间分布。尽管碰撞级联先前已被描述为分形,但其分形参数与辐射损伤累积的实验观察之间的相关性仍然难以捉摸。在这里,我们使用脉冲离子束方法研究在100 C下用不同质量的离子辐照的3C-SiC中的缺陷相互作用动力学。这些数据,连同先前对SiC和Si的研究结果,用辐射损伤形成模型进行了分析,该模型解释了碰撞级联的分形性质。我们的重点是从脉冲束测量中提取有效缺陷扩散长度。结果表明,对于Si和SiC,碰撞级联都是分形维数,其分形维数约为1-2,具体取决于离子质量,能量和距样品表面的深度。在我们的分形模型中,SiC的有效缺陷扩散长度为〜10 nm,Si的有效缺陷扩散长度为〜20 nm,并且随着级联密度的增加而减小。这些结果证明了碰撞级联的分形特性可以用来解释实验观察结果和预测材料对辐射的响应的通用方法。

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