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Quantifying Arctic lower stratospheric ozone sources in winter and spring

机译:量化冬季和春季北极平流层下层臭氧的来源

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摘要

The dynamical and chemical characteristics of unusually low Arctic ozone events in 2005 and 2011 have been well-studied. However, the quantitative identification of Arctic ozone sources is lacking. Here, we use tagged ozone tracers in a numerical simulation to quantify the contributions to Arctic lower stratospheric ozone (ARCLS_O3) at diverse latitudes in winter and spring from 2005–2011. We demonstrate that the northern mid-latitudinal stratosphere steadily contributes approximately half of ARCLS_O3. The absolute contributions during February have evident variations, which are smaller in cold years (151.3 ± 7.0 Dobson units (DU) in 2005 and 139.0 ± 7.4 DU in 2011) and greater in warm years (182.6 ± 7.3 DU in 2006 and 164.6 ± 7.4 DU in 2009). The tropical stratosphere is also an important source. During February, its absolute contributions are 66.5 ± 11.5 DU (2005), 73.1 ± 4.7 DU (2011), 146.0 ± 9.0 DU (2006), and 153.7 ± 7.0 DU (2009). Before and after stratospheric warming, variations in the tropical components of ARCLS_O3 (51.8 DU in 2006 and 77.0 DU in 2009) are significantly larger than those in the mid-latitudinal components (17.6 DU in 2006 and 18.1 DU in 2009). These results imply that although the mid-latitudinal components of ARCLS_O3 are larger, the tropical components control stratospheric temperature-induced ARCLS_O3 anomalies in winter and spring.
机译:对2005年和2011年异常低的北极臭氧事件的动力学和化学特征进行了深入研究。但是,缺乏对北极臭氧源的定量鉴定。在这里,我们在数字模拟中使用带标签的臭氧示踪剂,以量化2005-2011年冬季和春季在不同纬度对北极低平流层臭氧(ARCLS_O3)的贡献。我们证明了北中纬平流层稳定地贡献了大约ARCLS_O3的一半。 2月的绝对贡献有明显的变化,在寒冷年份较小(2005年为151.3±7.0道布森单位(DU),2011年为139.0±7.4 DU),而在温暖年份则更大(2006年为182.6±7.3 DU和164.6±7.4。 2009年DU)。热带平流层也是重要来源。在2月份,其绝对贡献为66.5±11.5 DU(2005),73.1±4.7 DU(2011),146.0±9.0 DU(2006)和153.7±7.0 DU(2009)。平流层变暖前后,ARCLS_O3的热带成分(2006年为51.8 DU,2009年为77.0 DU)的变化明显大于中纬度成分(2006年为17.6 DU,2009年为18.1 DU)。这些结果表明,尽管ARCLS_O3的中纬度分量较大,但热带分量控制了冬季和春季平流层温度引起的ARCLS_O3异常。

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