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Spin dynamics of the block orbital-selective Mott phase

机译:块轨道选择莫特相的自旋动力学

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摘要

Iron-based superconductors display a variety of magnetic phases originating in the competition between electronic, orbital, and spin degrees of freedom. Previous theoretical investigations of the multi-orbital Hubbard model in one-dimension revealed the existence of an orbital-selective Mott phase (OSMP) with block spin order. Recent inelastic neutron scattering (INS) experiments on the BaFe2Se3 ladder compound confirmed the relevance of the block-OSMP. Moreover, the powder INS spectrum revealed an unexpected structure, containing both low-energy acoustic and high-energy optical modes. Here we present the theoretical prediction for the dynamical spin structure factor within a block-OSMP regime using the density-matrix renormalization-group method. In agreement with experiments, we find two dominant features: low-energy dispersive and high-energy dispersionless modes. We argue that the former represents the spin-wave-like dynamics of the block ferromagnetic islands, while the latter is attributed to a novel type of local on-site spin excitations controlled by the Hund coupling.
机译:铁基超导体显示出各种磁相,这些磁相源于电子,轨道和自旋自由度之间的竞争。先前对多轨道Hubbard模型的一维理论研究表明,存在具有块自旋顺序的轨道选择性Mott相(OSMP)。最近在BaFe2Se3阶梯化合物上进行的非弹性中子散射(INS)实验证实了嵌段OSMP的重要性。此外,粉末INS光谱显示出意想不到的结构,既包含低能声学模式又包含高能光学模式。在这里,我们提出使用密度矩阵重归一化群方法对一个块OSMP机制内的动态自旋结构因子的理论预测。与实验一致,我们发现了两个主要特征:低能量色散和高能量色散模式。我们认为,前者代表了块状铁磁岛的自旋波状动力学,而后者则归因于由Hund耦合控制的新型局部现场自旋激发。

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