The General theory of Relativity (GR) brought gravity into accord with the principles of locality and relativity. Since its discovery it has been preeminent, recognized as the most accurate description of gravity on the many scales where it has been tested. During this period, seemingly radical predictions like the existence of black holes and the expansion of the Universe have been verified and testify to the great leap of insight that GR represented in our understanding of space and time. However not all precision observations of astrophysical systems have yielded easily to interpretation within GR, and with the discovery of cosmic acceleration, there is genuine concern that General Relativity may be incomplete when describing the Universe on the largest sizes imaginable.;In this uncertainty, many theoretical models have been proposed. In this thesis we shall first outline the motivation behind a certain subset of these models and the known issues that arise in interpreting these models as alternative theories of gravity. Then focus on one variety of theory the ƒ( R) modifications to gravity. Demonstrating that many of the known instabilities have a common origin and that they are avoided when treating these theories via perturbative constraints.;In the second part of this work we examine the astrophysical impact of modifications to gravity, first in the case of high mass neutron stars, then subsequently on corrections to the line profile of neutral hydrogen from violations of the equivalence principle. Finally we explore the phenomenology of modifications to gravity that produce late-Universe acceleration. In particular, what solutions are allowed and what range of accelerations are predicted as a result. Furthermore we explore how a correction to gravity at large scales would impact the growth and evolution of cosmological perturbations.
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