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Nonlinear optical response of Gd2@C80 thin films

机译:Gd2 @ C80薄膜的非线性光学响应

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Abstract: Single beam zscan experiments were carried out using a 130 fs tunable Ti:Sapphire-OPA laser system. The size and the sign of the third order susceptibility were measured at 400 nm, 590 nm, 648 nm, 800 nm, and 1000 nm. At 800 measurements were conducted for different pulse durations between 130 fs and 1 ps. Our results show that the measured values of the third order nonlinearity were relatively large, negative, and strongly dependent on pulse duration and wavelength. We found that, when wavelength and pulse duration are taken into account, the third order susceptibility of Gd$-2$/ at C$-80$/ is about one order of magnitude larger than that of empty-cage C$-60$/ or C$-70$/. !11
机译:摘要:使用130 fs可调谐Ti:Sapphire-OPA激光系统进行单光束zscan实验。在400 nm,590 nm,648 nm,800 nm和1000 nm处测量了三次磁化率的大小和符号。在800 fs下对130 fs和1 ps之间的不同脉冲持续时间进行了测量。我们的结果表明,三阶非线性的测量值相对较大,为负值,并且强烈依赖于脉冲持续时间和波长。我们发现,考虑到波长和脉冲持续时间,Gd $ -2 $ /在C $ -80 $ /时的三阶磁化率比空笼式C $ -60 $约大一个数量级。 /或C $ -70 $ /。 !11

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