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Study of Ozone Decomposition Using TiO_2-Graphene Composites

机译:使用TiO_2-石墨烯复合材料研究臭氧分解

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Graphene (Gn) were prepared by reduction of graphite oxide (GO), which was obtained from oxidation of graphite powder by a modified Hummers method. The composite of titanium dioxide/graphene (TiO_2/Gn) was synthesized using tetrabutyl titanate and GO as the precursors by a sol-gel method. The ozone photodecomposition efficiency of TiO_2/Gn was operated under ultraviolet-visible (UV-Vis, λ>365nm) light irradiation. Results showed that as-prepared TiO_2/Gn composite exhibited photodecomposition efficiency of 66.12% under UV-Vis light irradiation lh with the initial concentration of 0.150ppm-0.200ppm, preliminary larger than that of pure TiO_2 (25.95%), self-photolysis of ozone without photocatalysts (1.33%). The effects of initial concentration of ozone and photodecomposition mechanism were discussed.
机译:通过通过修饰的悍马方法还原从石墨粉末获得石墨氧化物(GO)来制备石墨烯(GN)。使用四丁酯合成二氧化钛/石墨烯(TiO_2 / GN)的复合物,通过溶胶 - 凝胶法作为前体。在紫外线可见(UV-VI,λ> 365nm)光照射下操作TiO_2 / GN的臭氧光致效率。结果表明,在UV-Vis光照射LH下,如制备的TiO_2 / GN复合材料在紫外线辐照下表现出66.12%的初始浓度为0.150ppm-0.200ppm,初步大于纯TiO_2(25.95%),自光解没有光催化剂的臭氧(1.33%)。讨论了臭氧和光分解机制初始浓度的影响。

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