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Effect of Microtubules Hierarchy on Photoinduced Hydrogen Generation and Application to Artificial Photosynthesis

机译:微管层次结构对人工光合作用的光致氢生成及其应用

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Several strategies have been explored from viewpoint of biomimetics to accomplish artificial photosynthesis by using macromolecules as a medium such as liposomes, supramolecules, and hydrogels. Differing from disordered solution systems in which multiple components such as photosensitizer and catalytic nanoparticle are diffusively mixed, the photochemical reactions occur efficiently in medium due to maintenance of the dipersibility of the components and specific molecular arrangement. Here we attempt to clarify the effect of medium hierarchy for photoinduced electronic transmission among multiple components. By conjugating each component on tubulin and integrating them via self-assembly to microtubules, ideal component arrangements with optimum distance for the electronic transmission will be possible.
机译:从生物体的观点来看,通过使用大分子作为脂质体,超分子和水凝胶等培养基来实现人造光合作用的几种策略。与脱敏剂如诸如光敏剂和催化纳米颗粒的多种组分的无序溶液系统不同,由于维持组分的偶像和特定分子布置,在培养基中有效地发生光化学反应。在这里,我们试图阐明媒体层次结构对多个组件之间的光导电子传输的影响。通过将每种组分缀合管蛋白并通过自组装将它们集成到微管中,可以实现具有最佳距离的理想部件布置。

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