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Stabilization of Néel order in frustrated magnets with increasing magnetic field

机译:随着磁场的挫折磁铁中Néel订单的稳定

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For low-dimensional frustrated quantum magnets, the dependence of the staggered moment m_s on a magnetic field is nonmonotonic: For small and intermediate fields, quantum fluctuations are gradually suppressed, leading to an increase of ms(H). For large applied magnetic fields however, the classically expected monotonous decrease is recovered. For the same reasons, the Néel ordering temperature T_N of such compounds first increases and then exhibits a reentrant behavior as a function of the field strength. The quantitative analysis of this behavior is an excellent tool to determine the frustration parameter of a given compound. We have derived a general linear spin-wave (LSW) theory in the presence of a magnetic field. Based on our LSW'theory, including a small interlayer coupling, we use a self-consistent approach determining T_N by the condition of a vanishing total moment. We apply our findings to the recently measured field dependence of the magnetic ordering temperature T_n of Cu(pz)_2(ClO_4)_2 in the framework of the S = 1/2 two-dimensional J_1-J_2 Heisenberg model. The observed increase with increasing field strength can be understood naturally using an intermediate frustration ratio J_2/J_1 ≈0.2, which is in accordance with the field dependence of the staggered moment.
机译:对于低维量子沮丧磁铁,在磁场中的交错的时刻M_S的依赖性是非单调的:对于小和中间字段,量子波动逐渐抑制,从而增加毫秒(H)。对于大型应用磁场然而,古典预计单调减少被回收。出于同样的原因,这样的化合物首先增加,然后所述尼尔有序温度T_N呈现折返行为的场强的函数。这种行为的定量分析是确定给定化合物的挫折参数的优秀工具。我们已得出在磁场的存在一般的线性自旋波(LSW)理论。根据我们LSW'theory,包括一个小的层间耦合,我们使用了一个自洽的方式确定T_N由总消失瞬间的状态。我们应用我们的发现为Cu(PZ)_2(ClO_4)_2在S的框架= 1/2二维J_1-J_2海森堡模型的磁有序温度T_n的最近测量字段依赖性。随着磁场强度的增加观察到的自然可以使用中间挫折比J_2 / J_1≈0.2,这是按照交错的时刻的场依赖性来理解。

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