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Effect of irradiation-induced micropores on fluorescence yield and radiation hardness of alkali-halide scintillation crystals

机译:辐照诱导的微孔对碱卤化物闪烁晶体荧光产率和辐射硬度的影响

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The analysis of experimental statistics, related to perfect CsI(Tl) crystals without impurities of oxygen radicals, shows that irradiation-induced variations in scintillation light output are mainly originated by the production of lattice defects capable of trapping electronic excitations. Below the nature of such irradiation-produced defects considered. It is shown that in the dose range of the order of 10 krad, where the known mechanisms of irradiation- induced changes are inefficient, the latter are originated by small pores growing under irradiation. Micropores affect scintillation yield even at low concentrations (approximately 10$+$MIN@7$/) due to a large section of exciton trapping exceeding the geometric section. The proposed model of growing micropores permits one to explain the observed does dependences of conversion efficiency and to use them for the control over the concentration of incipient micropores - a structural characteristic important for radiation stability.
机译:实验统计的分析与无氧自由基杂质的完美CSI(TL)晶体相关,表明闪烁光输出的照射诱导的变化主要由能够捕获电子激发的晶格缺陷的产生。低于这种辐照产生的缺陷的性质。结果表明,在10克拉德的剂量范围内,其中辐射诱导的变化的已知机制效率低下,后者源于照射下生长的小孔口。由于大部分Exciton捕获超过几何部分,微孔即使在低浓度(约10美元+售价@ 7 $ /)的情况下也会影响闪烁率。所提出的生长微孔模型允许人们解释观察到的转换效率的依赖性,并使用它们来控制初生微孔的浓度 - 对于辐射稳定性重要的结构特性。

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