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Fractals in microcavities: giant coupled, multiplicative enhancement of optical responses

机译:微腔的分形:巨型耦合,乘法增强光学响应

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Lasing at extremely low pump intensities, below 1 mW, and dramatically enhanced Raman scattering were observed for a novel class of optical materials, microcavities doped with nano-structured fractal aggregates. Nano-structured fractal aggregates lead to giant local-fields concentrated in "hot spots" much smaller in size than the size of the fractal and the wavelength. Coupling the localized plasmon modes in fractal aggregates with microcavity resonances further increases the local fields. These microcomposites possess unique optical characteristics, including extremely large probabilities of radiative processes. An extremely pronounced time-dependent lasing effect of dye molecules adsorbed on silver particles was also observed in oar experiment This time dependence is likely due to photo-stimulated aggregation of silver colloid particles and the gradient forces pulled fractal aggregates into the high-field area associated with the morphology-dependent resonance mode.
机译:在极低的泵强度下激光,低于1兆瓦,并针对新型光学材料进行了显着增强的拉曼散射,微腔掺杂有纳米结构分形聚集体。纳米结构的分形聚集体导致巨型局部尺寸小于分形和波长的大小小于“热点”。耦合具有微腔聚集体的局部化的等离子体模式与微腔共振进一步增加了局部场。这些微型复合材料具有独特的光学特性,包括极大的辐射过程概率。在OAR实验中也观察到吸附在银颗粒上的极其明显的时间依赖性激光效果在OAR实验中,这次依赖性可能是由于银胶体颗粒的光刺激聚集,并且梯度力将分形聚集体拉入相关的高场区域具有形态学相关的共振模式。

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