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EFFECTIVENESS OF A DOPANT IN U-ZR METALLIC FUEL TO PREVENT LANTHANIDE MIGRATION

机译:掺杂剂在U-ZR金属燃料中的有效性,以防止镧系元素迁移

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Advanced fast reactor concepts to achieve ultra-high burnup (~50%) without requiring refueling by way of using metallic alloy fuel have gained interest. Fission product lanthanide accumulation at high burnup is substantial and its migration to cladding and reaction with cladding is a potential life-limiting phenomenon. As a means to solve this problem, adding an element that forms stable compounds with lanthanides to immobilize them has been proposed. The theoretical assessment shows that indium, thallium, gallium, and antimony are good candidates. Except for Sb, because these elements are low-melting elements, liquid metal embrittlement of cladding is a concern if large sized agglomerates exist contacting the cladding. Alloy characterization of as-fabricated samples was performed to examine the effectiveness of the dopant addition method using optical microscopy and scanning electron microscophy.
机译:先进的快速反应堆概念实现超高燃烧(〜50%)而无需通过使用金属合金燃料获得感兴趣的方式进行加油。在高燃烧中的裂变产物镧系积累是实质性的,并且其与包层的迁移和包层的反应是潜在的寿命限制现象。作为解决该问题的手段,添加了形成稳定化合物的元素,以使它们固定它们。理论评估表明,铟,铊,镓和锑是良好的候选者。除了Sb,因为这些元素是低熔点元件,如果存在大尺寸的附聚物,则包层的液态金属脆化是一种问题,因为如果存在大型尺寸的聚集物,则存在与包层接触的大型尺寸附聚物。进行用光学显微镜和扫描电子显微镜检查掺杂剂添加方法的有效性的制造样品的合金表征。

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