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EFFECTIVENESS OF A DOPANT IN U-ZR METALLIC FUEL TO PREVENT LANTHANIDE MIGRATION

机译:U-Zr金属燃料中掺杂剂对镧系元素迁移的抑制作用

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Advanced fast reactor concepts to achieve ultra-high burnup (~50%) without requiring refueling by way of using metallic alloy fuel have gained interest. Fission product lanthanide accumulation at high burnup is substantial and its migration to cladding and reaction with cladding is a potential life-limiting phenomenon. As a means to solve this problem, adding an element that forms stable compounds with lanthanides to immobilize them has been proposed. The theoretical assessment shows that indium, thallium, gallium, and antimony are good candidates. Except for Sb, because these elements are low-melting elements, liquid metal embrittlement of cladding is a concern if large sized agglomerates exist contacting the cladding. Alloy characterization of as-fabricated samples was performed to examine the effectiveness of the dopant addition method using optical microscopy and scanning electron microscophy.
机译:先进的快速反应堆概念可以实现超高燃耗(〜50%),而无需使用金属合金燃料进行加油。裂变产物镧系元素在高燃耗下会大量积累,并且其向包层的迁移以及与包层的反应是潜在的限制寿命的现象。作为解决该问题的手段,已经提出了添加与镧系元素形成稳定化合物以使其固定化的元素。理论评估表明,铟,th,镓和锑是不错的选择。除了Sb外,由于这些元素是低熔点元素,因此如果存在大尺寸的团聚体,则覆盖层的液态金属脆化将成为一个问题。使用光学显微镜和扫描电子显微镜对制成的样品进行合金表征,以检查掺杂剂添加方法的有效性。

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