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Ultrafast dynamics of confined and localized excitons in low-dimensional semiconductors

机译:低维半导体中局域和局域激子的超快动力学

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Abstract: Coherent optical spectroscopy in the form of nonlinear transient four-wave mixing (TFWM) and linear resonant Rayleigh scattering (RRS) has been applied to investigate the exciton dynamics of low-dimensional semiconductor heterostructures. The dephasing times of excitons are determined from the decay of the spectrally resolved non- linear signal as a function of the delay between the incident pulses in a two-beam TFWM experiment, and from the real time analysis of single speckles in RRS experiments (pure dephasing). From the density- and temperature- dependence of the dephasing times the exciton-exciton and the exciton-phonon interactions are determined. The degree of coherence of the secondary emission is determined from the speckle analysis.!20
机译:摘要:以非线性瞬态四波混频(TFWM)和线性共振瑞利散射(RRS)形式的相干光谱研究了低维半导体异质结构的激子动力学。激子的移相时间取决于频谱分辨的非线性信号的衰减与两光束TFWM实验中入射脉冲之间的延迟之间的函数关系,以及RRS实验中对单个散斑的实时分析(纯移相)。根据相移时间的密度和温度依赖性,确定激子-激子和激子-声子相互作用。通过散斑分析确定二次发射的相干度!20

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