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Optical two-dimensional coherent spectroscopy of semiconductor nanostructures

机译:半导体纳米结构的二维二维相干光谱

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Our recent work on optical two-dimensional coherent spectroscopy (2DCS) of semiconductor materials is reviewed. We present and compare two approaches that are appropriate for the study of semiconductor nanostructures. The first one is based on a non-collinear geometry, where the Four-Wave-Mixing (FWM) signal is detected in the form of a radiated optical field. This approach works for samples with translational symmetry, such as Quantum Wells (QWs), or large and dense ensembles of Quantum Dots (QDs). The second method is based on a collinear geometry, where the FWM is detected in the form of a photocurrent. This second approach enables 2DCS of samples where translational symmetry is broken, such as single QDs, nanowires, or nanotubes, and small ensembles thereof. For each method, we provide an example of experimental results obtained on semiconductor QWs. In particular, it is shown how 2DCS can reveal coherent excitonic coupling between adjacent QWs.
机译:我们对半导体材料的光学二维相干光谱学(2DCS)的最新工作进行了回顾。我们提出并比较了两种适用于研究半导体纳米结构的方法。第一个基于非共线几何形状,其中以辐射光场的形式检测四波混频(FWM)信号。这种方法适用于具有平移对称性的样品,例如量子阱(QW)或大而密集的量子点集合(QD)。第二种方法基于共线几何,其中以光电流的形式检测FWM。第二种方法使2DCS样品的翻译对称性破裂,例如单个QD,纳米线或纳米管及其小集合。对于每种方法,我们提供了一个在半导体QW上获得的实验结果的示例。特别是,它显示了2DCS如何揭示相邻QW之间的相干激子耦合。

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