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A Carbide Catalyst Effective for the Dry Reforming of Methane at Atmospheric Pressure

机译：大气压下甲烷干法重整的硬质合金催化剂

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摘要

A catalyst composed of metallic nickel and molybdenum carbide has been fabricated for CO_2 reforming of CH_4. Aspects concerning the formation of Ni and Mo_2C, their synergistic effects for CH_4 and CO_2 activation, and the establishment of a redox cycle were studied. Due to the catalytic oxidation-recarburization cycle, the Ni-Mo_2C catalyst is superior to the traditional metal carbide catalysts as verified by its stable activity in the dry reforming of CH_4 at atomspheric pressure.
机译：制备了由金属镍和碳化钼组成的催化剂，用于CH_2的CO_2重整。研究了Ni和Mo_2C的形成，它们对CH_4和CO_2活化的协同作用以及氧化还原循环的建立。 Ni-Mo_2C催化剂由于具有催化氧化-再碳化循环的能力，因此在传统的金属碳化物催化剂上具有优异的活性，这是由于其在常压下CH_4的干重整中具有稳定的活性所证实的。

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  • 来源
  • 会议地点 Washington DC(US);Washington DC(US)
  • 作者

    Jun Guo; An-Jie Zhang; Ai-Min Zhu; Yong Xu; C. T. Au; Chuan Shi;

  • 作者单位

    Laboratory of Plasma Physical Chemistry, Dalian University of Technology,Dalian, PR China;

    Laboratory of Plasma Physical Chemistry, Dalian University of Technology,Dalian, PR China;

    Laboratory of Plasma Physical Chemistry, Dalian University of Technology,Dalian, PR China;

    Laboratory of Plasma Physical Chemistry, Dalian University of Technology,Dalian, PR China;

    Department of Chemistry, Hong Kong Baptist University,Kowloon Tong, Hong Kong;

    Laboratory of Plasma Physical Chemistry, Dalian University of Technology,Dalian, PR China,State Key Laboratory of the Fine Chemicals,Dalian University of Technology, Dalian, PR China;

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  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类 二氧化碳的生产;
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