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Cerium-modified manganese octahedral molecular sieves as catalysts for selective catalytic reduction
Cerium-modified manganese octahedral molecular sieves as catalysts for selective catalytic reduction
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机译:铈改性的锰八面体分子筛作为催化剂的选择性催化还原
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摘要
Catalysts and articles useful for selective catalytic reduction (SCR) are disclosed. The catalyst comprises a cerium oxide and an octahedral molecular sieve (OMS) comprising manganese oxide. The catalysts, which comprise 0.1 to 50 wt. % of cerium, can be made by doping, ion-exchange, deposition, or other techniques. Also disclosed is an SCR process in which a gaseous mixture comprising nitrogen oxides is selectively reduced in the presence of a reductant and the cerium-modified OMS catalyst. The cerium-modified manganese oxide OMS catalysts offer unexpected advantages for selective catalytic reduction, especially NH3-SCR, including improved thermal stability and improved activity for NOx conversion, especially at relatively low temperatures (100° C. to 250° C.).
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