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Time-delayed four-wave mixing: the interplay between laser field fluctuations and the atomic memory time

机译:延时四波混频:激光场波动与原子记忆时间之间的相互作用

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摘要

Coherent signals induced by fundamentally incoherent phenomena through a four-wave mixing process are among the most intriguing and subtle effects in nonlinear spectroscopy. These effects were initially observed by Bloembergen and his co-workers in the form of pressure-induced extra resonances in four-wave mixing. Using standard perturbance techniques based on the optical Bloch equations, they suggested that these collision induced resonances were the result of a "destruction of the destructive interference" existent between two alternate time-ordered pathways. Subsequently, Prior et al realised that fluctuations in the incident radiation fields could play essentially the same role as the collisionally induced dephasing. In practice, of course, both collisional dephasing and field fluctuations are present in a typical atomic vapor pulsed four-wave mixing experiment. If the timescales governing these two effects approach one another, one can expect to gain valuable new insight into this fascinating process of "incoherently" inducing a coherent signal
机译:通过四波混频过程从根本上不相干的现象中感应出的相干信号是非线性光谱学中最引人入胜和最微妙的影响之一。这些影响最初是由Bloembergen及其同事以四波混频中压力引起的额外共振的形式观察到的。他们使用基于光学Bloch方程的标准摄动技术,认为这些碰撞引起的共振是两个替代时间顺序路径之间存在“破坏性干扰破坏”的结果。随后,Prior等人意识到入射辐射场中的波动起着与碰撞引起的相移基本相同的作用。当然,实际上,在典型的原子蒸气脉冲四波混合实验中,会出现相移和相场波动。如果控制这两种效应的时间尺度彼此接近,那么人们可以期望对这种“非相干”地产生相干信号的迷人过程获得有价值的新见解。

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