Magnetic hysteresis loops in molecular-based magnetic materials AFe(II)Fe(III)(C2O4)(3)

摘要

A molecular-based magnetic material AFe(II)Fe(III)(C2O4)(3) (A = organic cation) with a honeycomb structure is studied. The molecular-based magnet system consists of mixed spin-2 and spin-5/2 honeycomb lattices with ferrimagnetic interlayer coupling. The magnetization, hysteresis loops and initial susceptibility have been calculated using a numerical method which includes both the longitudinal and transverse fields. We investigated the magnetic reversal of the system and found the existence of triple hysteresis loop patterns, affected by the anisotropy, longitudinal and transverse fields, and interlayer and intralayer exchange.