Transverse and in-plane modification of superconductivity and electronic structure in the quasi-two-dimensional organic conductor kappa-(BEDT-TTF)(2) Cu(SCN)(2) by uniaxial stress

摘要

We have employed uniaxial stress along the principal axes of the quasi-two-dimensional organic superconductor kappa-(BEDT-TTF)(2)Cu(SCN)(2) (BEDT-TTF = bis(ethylenedithio)tetrathiafulvalene). The lattice anisotropy is there by altered, with corresponding changes in the intermolecular transfer energies. The effect of uniaxial stress on the superconducting transition temperature T-c and critical field B-c2 is found to be anisotropic. There is an indication of an increase in T-c and an increase in B-c2 for in-plane stress, but both parameters decrease rapidly for transverse (interplane) stress. Magnetotransport studies reveal stress-induced changes in the Fermi surface through the observation of the Shubnikov-de Haas oscillations. The stress dependence of a resistive anomaly in the magnetoresistance, which is associated with the critical field B-c2 is also investigated. We discuss the experimental findings in the context of recent phenomenological and theoretical treatments of quasi-two-dimensional systems where the anisotropic triangular-lattice Hubbard model has been used to treat two-dimensional superconductors. [References: 30]