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Transient Interband Light Absorption by Quantum Dots: Nondegenerate Case of Pump-Probe Spectroscopy

机译:量子点的瞬态带间光吸收:泵浦探针光谱的非退化情况

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摘要

A theoretical description of the pump-probe optical method is presented that is adapted to semiconductor quantum dots and makes it possible to determine the energy relaxation rates of the excited states of electron-hole pairs and excitons in these objects. A scheme of the method is considered in which the carrier frequencies of optical pump and probe pulses are close to the resonance with different interband transitions of the quantum-dot electron subsystem (nondegenerate case). It is assumed that the final states to which electron subsystem passes as a result of the absorption of pump and probe pulses are interrelated by intraband relaxation. The probe-pulse energy absorption induced by the pump pulse is analyzed as a function of the delay time between the pulses. It is shown that this dependence tends to be biexponential under certain conditions. The exponential factors are proportional to the energy relaxation rates of the resonantly excited states of electron-hole pairs and excitons, while the preexponential factors depend on the intraband relaxation rate.
机译:提出了泵浦探针光学方法的理论描述,该方法适用于半导体量子点,并可以确定这些对象中电子-空穴对和激子的激发态的能量弛豫率。考虑该方法的方案,其中光泵和探针脉冲的载波频率接近于量子点电子子系统的不同带间跃迁的谐振(非简并的情况)。假定由于泵浦和探针脉冲的吸收而使电子子系统通过的最终状态通过带内弛豫相互关联。由泵浦脉冲引起的探测脉冲能量吸收将根据脉冲之间的延迟时间进行分析。结果表明,在某些条件下,这种依赖性趋于双指数。指数因子与电子-空穴对和激子的共振激发态的能量弛豫速率成正比,而预指数因子则取决于带内弛豫速率。

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