Integration of methanol steam reforming and combustion in a microchannel reactor for H2 production: A CFD simulation study

摘要

A computational fluid dynamics (CFD) study of the thermal integration of the steam reforming of methanol (SRM) and the combustion of methanol in a catalytic microchannel reactor is presented. This issue is of interest for in situ H2 production for portable power units based on low-temperature PEM fuel cells. Three-dimensional simulations have been carried out under relevant conditions for the SRM reaction that have shown that microreactors allow achieving complete methanol reforming and combustion at space velocities as high as 50,000 h~(-1) with selectivities for H2 above 99% at relatively low temperatures in the 270-290 °C range.