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Ultrafast observation of critical nematic fluctuations and giant magnetoelastic coupling in iron pnictides

机译:超快速观测铁的临界向列波动和巨大的磁弹性耦合

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Many of the iron pnictides have strongly anisotropic normal-state characteristics, important for the exotic magnetic and superconducting behaviour these materials exhibit. Yet, the origin of the observed anisotropy is unclear. Electronically driven nematicity has been suggested, but distinguishing this as an independent degree of freedom from magnetic and structural orders is difficult, as these couple together to break the same tetragonal symmetry. Here we use time-resolved polarimetry to reveal critical nematic fluctuations in unstrained Ba(Fe-1-Co-x(x))(2)As-2. The femtosecond anisotropic response, which arises from the two-fold in-plane anisotropy of the complex refractive index, displays a characteristic two-step recovery absent in the isotropic response. The fast recovery appears only in the magnetically ordered state, whereas the slow one persists in the paramagnetic phase with a critical divergence approaching the structural transition temperature. The dynamics also reveal a gigantic magnetoelastic coupling that far exceeds electron-spin and electron-phonon couplings, opposite to conventional magnetic metals.RI Canfield, Paul/H-2698-2014; Fernandes, Rafael/E-9273-2010
机译:许多铁肽具有强烈的各向异性常态特性,这对于这些材料表现出的奇特的磁性和超导行为很重要。然而,所观察到的各向异性的起源尚不清楚。已经提出了电子驱动的向列性,但是很难将其作为独立的自由度与磁性和结构顺序区分开来,因为它们耦合在一起以破坏相同的四边形对称性。在这里,我们使用时间分辨极化仪揭示未应变的Ba(Fe-1-Co-x(x))(2)As-2中的临界向列波动。飞秒各向异性响应是由复数折射率的两倍平面内各向异性引起的,显示出各向同性响应中不存在的特征性两步恢复。快速恢复仅在磁性有序状态下出现,而慢速恢复则在顺磁相中持续存在,并且临界发散接近结构转变温度。动力学还揭示了巨大的磁弹性耦合,其远远超过了电子自旋和电子-声子耦合,与传统的磁性金属相反。RICanfield,Paul / H-2698-2014;费尔南德斯,拉斐尔/ E-9273-2010

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