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Low-temperature electronic transport in single K0.27MnO2 center dot 0.5H(2)O nanowires: enhanced electron-electron interaction

机译:单根K0.27MnO2中心点0.5H(2)O纳米线中的低温电子传输:增强的电子-电子相互作用

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摘要

The current-voltage (I-V) characteristics and electrical resistivity of isolated potassium manganese oxide (K0.27MnO2 center dot 0.5H(2)O) nanowires prepared by a simple hydrothermal method were investigated over a wide temperature range from 300 to 4 K. With lowering temperature, a transition from linear to nonlinear I-V curves was observed around 50 K, and a clear zero bias anomaly (i.e., Coulomb gap-like structure) appeared on the differential conductance (dI/dV) curves, possibly due to enhanced electron-electron interaction at low temperatures. The temperature dependence of resistivity, ln rho alpha T-1/2, follows the Efros-Shklovskii (ES) law, as expected in the presence of a Coulomb gap. Here we note that both the ES law and Coulomb blockade can in principle lead to a reduced zero bias conductance at low temperatures; in this study we cannot exclude the possibility of Coulomb-blockade transport in the measured nanowires, especially in the low-temperature range. It is still an open question how to pin down the origin of the observed reduction to a Coulomb gap (ES law) or Coulomb blockade.
机译:在300至4 K的宽温度范围内,研究了通过简单的水热法制备的离体的氧化钾锰氧化物(K0.27MnO2中心点0.5H(2)O)纳米线的电流-电压(IV)特性和电阻率。降低温度时,在50 K左右观察到了从线性IV曲线到非线性IV曲线的过渡,并且在微分电导(dI / dV)曲线上出现了清晰的零偏压异常(即库仑间隙状结构),这可能是由于电子的增强引起的。低温下的电子相互作用。电阻率的温度依赖性(ln rhoαT-1 / 2)遵循Efros-Shklovskii(ES)定律,这是在存在库仑间隙的情况下所预期的。这里我们注意到,ES律和库仑封锁原则上都可以导致低温下零偏电导的降低;在这项研究中,我们不能排除在测得的纳米线中库仑阻塞转运的可能性,尤其是在低温范围内。如何将观察到的减少的源头确定为库仑缺口(ES法)或库仑封锁仍然是一个悬而未决的问题。

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