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Preparation and evaluation of a metallic foam catalyst for steam-CO2 reforming of methane in GTL-FPSO process

机译:GTL-FPSO工艺中用于甲烷蒸汽-CO2重整的金属泡沫催化剂的制备和评价

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摘要

A metallic foam catalyst was used to improve the heat transfer of a reactor for the steam-CO2 reforming (SCR) of methane in the GTL-FPSO (gas to liquid-floating production storage and offloading) process. The metallic foam catalyst was prepared and examined by scanning electron microscopy, fall-off test and SCR reaction. The radial heat transfer was characterized in terms of the Nusselt number and was compared with the pellet catalyst to confirm the improvement in the heat transfer of the metallic foam catalyst As a result of the fall-off test, the adhesion strength was highest at an Al2O3/AIP molar ratio of 5. The Nusselt number of the metallic foam catalyst was higher than that of the conventional pellet catalyst Therefore, the reformer had a uniform temperature distribution along the catalyst-bed when the metallic foam catalyst was used.
机译:使用金属泡沫催化剂改善了GTL-FPSO(气液浮选产品存储和卸载)过程中甲烷的蒸汽CO2重整(SCR)反应器的传热。制备金属泡沫催化剂,并通过扫描电子显微镜,脱落试验和SCR反应进行检查。径向传热用Nusselt数表征,并与粒状催化剂进行比较,以确认金属泡沫催化剂的传热有所改善。脱落试验的结果是,Al2O3的附着强度最高/ AIP摩尔比为5。金属泡沫催化剂的努塞尔数高于常规粒状催化剂的努塞尔数。因此,当使用金属泡沫催化剂时,重整器沿催化剂床的温度分布均匀。

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