Contribution of regional sources to atmospheric methane over the Amazon Basin in 2010 and 2011

摘要

We present an assessment of methane (CH4) atmospheric concentrations over the Amazon Basin for 2010 and 2011 using a 3-D atmospheric chemical transport model, two wetland emission models, and new observations made during biweekly flights made over four locations within the basin. We attempt to constrain basin-wide CH4 emissions using the observations, and since 2010 was an unusually dry year, we assess the effect of this drought on Amazonian methane emissions. We find that South American emissions contribute up to 150 ppb to concentrations at the sites, mainly originating from within the basin. Our atmospheric model simulations agree reasonably well with measurements at three of the locations (0.28 <= r(2) <= 0.63, mean bias <= 9.5 ppb). Attempts to improve the simulated background CH4 concentration through analysis of simulated and observed sulphur hexafluoride concentrations do not improve the model performance, however. Through minimisation of seasonal biases between the simulated and observed atmospheric concentrations, we scale our prior emission inventories to derive total basin-wide methane emissions of 36.5-41.1 Tg(CH4)/yr in 2010 and 31.6-38.8 Tg(CH4)/yr in 2011. These totals suggest that the Amazon contributes significantly (up to 7%) to global CH4 emissions. Our analysis indicates that factors other than precipitation, such as temperature variations or tree mortality, may have affected microbial emission rates. However, given the uncertainty of our emission estimates, we cannot say definitively whether the noncombustion emissions from the region were different in 2010 and 2011, despite contrasting meteorological conditions between the two years.