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Why does surface ozone peak before a typhoon landing in southeast China?

机译:为什么在台风登陆中国东南之前,地表臭氧达到峰值?

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A high O-3 episode with the large increases in surface ozone by 21-42 ppbv and the nocturnal surface O-3 levels exceeding 70 ppbv was observed in the region between Xiamen and Quanzhou over the southeastern coast of China during 12-14 June 2014, before the Typhoon Hagibis landing. Variations in the surface O-3, NO2, CO and meteorology during the Typhoon Hagibis event clearly suggest a substantial impact of the peripheral downdrafts in the large-scale typhoon circulation on such an O-3 episode excluding the contributions of photochemical production and the horizontal transport. The influence of vertical O-3 transport from the upper troposphere and lower stratosphere (UTLS) region on high surface O-3 levels is further confirmed by a negative correlation between surface O-3 and CO concentrations as well as dry surface air observed during the O-3 episode. This study provides observational evidence of typhoon-driven intrusion of O-3 from the UTLS region to surface air, revealing a significant effect of such a process of stratosphere-troposphere exchange (STE) of O-3 on tropospheric O-3 and ambient air quality.
机译:2014年6月12日至14日,在中国东南沿海的厦门和泉州之间,观测到O-3高度升高,表面臭氧大量增加21-42 ppbv,夜间O-3水平超过70 ppbv。 ,在台风哈吉比斯登陆之前。台风哈吉比事件期间表面O-3,NO2,CO和气象学的变化清楚地表明,大规模台风环流的外围下降气流对这种O-3事件具有重大影响,但不包括光化学生产和水平方向的影响。运输。来自高对流层和低平流层(UTLS)区域的垂直O-3运移对高表面O-3含量的影响进一步得到了确认,这是由于表面O-3和CO浓度以及在观测期间观测到的干燥地面空气之间存在负相关关系。 O-3集。这项研究提供了台风驱动的O-3从UTLS区域侵入地面空气的观测证据,揭示了O-3的平流层-对流层交换(STE)对对流层O-3和环境空气的这种显着影响质量。

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